A Centimeter-Sized Quaternary Ti-Zr-Be-Ag Bulk Metallic Glass

<table class="table-group" id="tab1"><tr><td><table class="table"><tr><td class="thead-hr" colspan="8"><hr/></td></tr><tr class="thead"><td align="left">Composition (at.%)</td><td align="center"><svg height="18.799999" id="M16" style="vertical-align:-4.77652pt" version="1.1" viewbox="0 0 18.8375 18.799999" width="18.8375" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
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t37 -4h417q23 0 33.5 5t25.5 21h23z" id="x1D447"></path></g>
<g transform="matrix(.012,-0,0,-.012,11.388,15.638)"><path d="M546 430q-14 -33 -37.5 -140t-38.5 -209q-29 -195 -156 -289q-29 -21 -70 -37t-78 -16q-62 0 -102.5 37t-40.5 69q0 27 26 48q19 15 25 -3q13 -43 46.5 -69t87.5 -26q55 0 83 21q29 22 50 65t43 140q14 64 29 163h-2q-55 -81 -149 -152q-59 -44 -102 -44q-23 0 -43.5 30
t-20.5 85q0 74 32.5 145.5t84.5 117.5q40 35 100 58.5t117 23.5q21 0 65 -8q30 -6 44 -6zM456 386q-40 16 -81 16q-29 0 -64 -13q-42 -17 -85 -97q-19 -36 -31.5 -86t-12.5 -86q0 -64 30 -64q20 0 52.5 21t60.5 52q74 81 95 123q26 62 36 134z" id="x1D454"></path></g>
</svg> (K)</td><td align="center"><svg height="15.8375" id="M17" style="vertical-align:-3.21404pt" version="1.1" viewbox="0 0 18.725 15.8375" width="18.725" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.55)"><path d="M649 676l-22 -187l-33 -2q3 56 -12 94q-8 20 -31.5 26.5t-86.5 6.5h-74l-90 -491q-4 -23 -6 -36.5t1 -25t7 -16.5t18 -9t27 -5t41 -3l-6 -28h-286l4 28q68 5 84 18.5t28 76.5l94 491h-55q-74 0 -100.5 -6t-41.5 -23q-24 -29 -54 -98l-32 1q32 98 53 188h22q7 -18 15 -22
t37 -4h417q23 0 33.5 5t25.5 21h23z" id="x1D447"></path></g>
<g transform="matrix(.012,-0,0,-.012,11.388,15.637)"><path d="M536 404q0 -17 -13.5 -31.5t-26.5 -14.5q-8 0 -15 10q-11 14 -25 14q-22 0 -67 -50q-47 -52 -68 -82l37 -102q31 -88 55 -88t78 59l16 -23q-32 -48 -68.5 -78t-65.5 -30q-19 0 -37.5 20t-29.5 53l-41 116q-72 -106 -114.5 -147.5t-79.5 -41.5q-21 0 -34.5 14t-13.5 37
q0 16 13.5 31.5t28.5 15.5q12 0 17 -11q5 -10 25 -10q22 0 57.5 36t89.5 111l-40 108q-22 58 -36 58q-21 0 -67 -57l-19 20q81 107 125 107q17 0 30 -22t39 -88l22 -55q68 92 108.5 128.5t74.5 36.5q20 0 32.5 -14t12.5 -30z" id="x1D465"></path></g>
</svg> (K)</td><td align="center"><svg height="15.8375" id="M18" style="vertical-align:-3.21404pt" version="1.1" viewbox="0 0 29.612499 15.8375" width="29.612499" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.55)"><path d="M600 0h-557v24l268 633l28 8l261 -641v-24zM497 50l-194 489l-196 -489h390z" id="x394"></path></g><g transform="matrix(.017,-0,0,-.017,10.959,11.55)"><path d="M649 676l-22 -187l-33 -2q3 56 -12 94q-8 20 -31.5 26.5t-86.5 6.5h-74l-90 -491q-4 -23 -6 -36.5t1 -25t7 -16.5t18 -9t27 -5t41 -3l-6 -28h-286l4 28q68 5 84 18.5t28 76.5l94 491h-55q-74 0 -100.5 -6t-41.5 -23q-24 -29 -54 -98l-32 1q32 98 53 188h22q7 -18 15 -22
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<g transform="matrix(.012,-0,0,-.012,22.275,15.637)"><path d="M536 404q0 -17 -13.5 -31.5t-26.5 -14.5q-8 0 -15 10q-11 14 -25 14q-22 0 -67 -50q-47 -52 -68 -82l37 -102q31 -88 55 -88t78 59l16 -23q-32 -48 -68.5 -78t-65.5 -30q-19 0 -37.5 20t-29.5 53l-41 116q-72 -106 -114.5 -147.5t-79.5 -41.5q-21 0 -34.5 14t-13.5 37
q0 16 13.5 31.5t28.5 15.5q12 0 17 -11q5 -10 25 -10q22 0 57.5 36t89.5 111l-40 108q-22 58 -36 58q-21 0 -67 -57l-19 20q81 107 125 107q17 0 30 -22t39 -88l22 -55q68 92 108.5 128.5t74.5 36.5q20 0 32.5 -14t12.5 -30z" id="x1D465"></path></g>
</svg> (K)</td><td align="center"><svg height="15.8375" id="M19" style="vertical-align:-3.22282pt" version="1.1" viewbox="0 0 15.275 15.8375" width="15.275" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.55)"><path d="M649 676l-22 -187l-33 -2q3 56 -12 94q-8 20 -31.5 26.5t-86.5 6.5h-74l-90 -491q-4 -23 -6 -36.5t1 -25t7 -16.5t18 -9t27 -5t41 -3l-6 -28h-286l4 28q68 5 84 18.5t28 76.5l94 491h-55q-74 0 -100.5 -6t-41.5 -23q-24 -29 -54 -98l-32 1q32 98 53 188h22q7 -18 15 -22
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<g transform="matrix(.012,-0,0,-.012,11.388,15.637)"><path d="M238 681l-124 -585q-7 -31 4 -31q10 0 37.5 18.5t49.5 41.5l16 -22q-40 -48 -89.5 -81.5t-76.5 -33.5q-42 0 -16 122l105 488q7 32 0 41t-39 9h-35l5 26q35 3 71 13t58 17.5t26 7.5q14 0 8 -31z" id="x1D459"></path></g>
</svg> (K)</td><td align="center"><i>T </i><sub>
                  rg</sub> = <svg height="18.799999" id="M20" style="vertical-align:-4.77652pt" version="1.1" viewbox="0 0 18.8375 18.799999" width="18.8375" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.55)"><path d="M649 676l-22 -187l-33 -2q3 56 -12 94q-8 20 -31.5 26.5t-86.5 6.5h-74l-90 -491q-4 -23 -6 -36.5t1 -25t7 -16.5t18 -9t27 -5t41 -3l-6 -28h-286l4 28q68 5 84 18.5t28 76.5l94 491h-55q-74 0 -100.5 -6t-41.5 -23q-24 -29 -54 -98l-32 1q32 98 53 188h22q7 -18 15 -22
t37 -4h417q23 0 33.5 5t25.5 21h23z" id="x1D447"></path></g>
<g transform="matrix(.012,-0,0,-.012,11.388,15.638)"><path d="M546 430q-14 -33 -37.5 -140t-38.5 -209q-29 -195 -156 -289q-29 -21 -70 -37t-78 -16q-62 0 -102.5 37t-40.5 69q0 27 26 48q19 15 25 -3q13 -43 46.5 -69t87.5 -26q55 0 83 21q29 22 50 65t43 140q14 64 29 163h-2q-55 -81 -149 -152q-59 -44 -102 -44q-23 0 -43.5 30
t-20.5 85q0 74 32.5 145.5t84.5 117.5q40 35 100 58.5t117 23.5q21 0 65 -8q30 -6 44 -6zM456 386q-40 16 -81 16q-29 0 -64 -13q-42 -17 -85 -97q-19 -36 -31.5 -86t-12.5 -86q0 -64 30 -64q20 0 52.5 21t60.5 52q74 81 95 123q26 62 36 134z" id="x1D454"></path></g>
</svg><i>/ </i><svg height="15.8375" id="M21" style="vertical-align:-3.22282pt" version="1.1" viewbox="0 0 15.275 15.8375" width="15.275" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.55)"><path d="M649 676l-22 -187l-33 -2q3 56 -12 94q-8 20 -31.5 26.5t-86.5 6.5h-74l-90 -491q-4 -23 -6 -36.5t1 -25t7 -16.5t18 -9t27 -5t41 -3l-6 -28h-286l4 28q68 5 84 18.5t28 76.5l94 491h-55q-74 0 -100.5 -6t-41.5 -23q-24 -29 -54 -98l-32 1q32 98 53 188h22q7 -18 15 -22
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<g transform="matrix(.012,-0,0,-.012,11.388,15.637)"><path d="M238 681l-124 -585q-7 -31 4 -31q10 0 37.5 18.5t49.5 41.5l16 -22q-40 -48 -89.5 -81.5t-76.5 -33.5q-42 0 -16 122l105 488q7 32 0 41t-39 9h-35l5 26q35 3 71 13t58 17.5t26 7.5q14 0 8 -31z" id="x1D459"></path></g>
</svg></td><td align="center"><span style="width: 8.6374998px;"><svg height="12.175" id="M22" style="vertical-align:-2.34499pt" version="1.1" viewbox="0 0 8.6374998 12.175" width="8.6374998" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,7.675)"><path d="M478 372q0 -39 -31 -97t-61 -98t-78 -98q-45 -55 -73 -102q-13 -79 -13 -197q-11 -11 -43.5 -25.5t-53.5 -15.5l-15 17q5 35 26 101.5t47 123.5q8 72 -1.5 174.5t-37.5 178.5q-14 37 -29 37q-20 0 -67 -65l-25 21q37 60 73 90.5t63 30.5q47 0 72 -112q13 -56 17.5 -141.5
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</svg></span></td><td align="center"><svg height="15.4" id="M23" style="vertical-align:-3.22282pt" version="1.1" viewbox="0 0 36.962502 15.4" width="36.962502" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.112)"><path d="M780 372q0 -191 -178 -297q-128 -75 -335 -75h-250l7 27q61 7 77 22t28 76l77 398q11 62 0 76.5t-77 22.5l6 28h292q164 0 258.5 -67.5t94.5 -210.5zM678 375q0 119 -73 180.5t-201 61.5q-62 0 -82 -13q-17 -7 -25 -53l-80 -427q-8 -47 -4 -62t26 -20q24 -6 80 -6
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<g transform="matrix(.012,-0,0,-.012,13.712,15.187)"><path d="M797 0h-214v26q46 5 58 17.5t12 63.5v167q0 116 -88 116q-48 0 -112 -52q3 -18 3 -42v-195q0 -46 11 -58t53 -17v-26h-214v26q48 5 59.5 17t11.5 60v172q0 115 -88 115q-47 0 -109 -52v-235q0 -47 10 -59.5t48 -17.5v-26h-211v26q50 5 62.5 17t12.5 60v207q0 48 -9 59.5
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</svg> (mm)</td></tr><tr><td class="thead-hr" colspan="8"><hr/></td></tr><tr><td align="left">Ti<sub>41</sub>Zr<sub>25</sub>Be<sub>34</sub> [<a href="/journals/amse/2014/192187/#B6">6</a>]</td><td align="center">607</td><td align="center">656</td><td align="center">49</td><td align="center">1123</td><td align="center">0.5405</td><td align="center">0.3792</td><td align="center"><span style="width: 21.1px;"><svg height="11.5125" id="M24" style="vertical-align:-0.17555pt" version="1.1" viewbox="0 0 21.1 11.5125" width="21.1" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.25)"><path d="M488 658v-28q-47 -3 -58.5 -12t-11.5 -39q49 -2 97 -15t93.5 -39.5t73.5 -75t28 -112.5q0 -53 -19.5 -96.5t-50 -71t-70 -47t-77.5 -27.5t-75 -9q0 -36 11.5 -45.5t58.5 -12.5v-28h-223v28q47 3 58.5 12.5t11.5 45.5q-47 1 -94.5 14t-93 39.5t-74.5 76t-29 114.5
q0 51 19 93.5t49 70t69.5 47t77.5 28t76 10.5q0 30 -11 39t-54 12v28h218zM335 118v429q-34 -2 -67 -13.5t-63.5 -35t-49.5 -65.5t-19 -96q0 -56 18.5 -99t49 -67.5t63.5 -37.5t68 -15zM418 547v-429q35 2 67.5 14t63.5 35.5t50 66.5t19 99t-19 99t-50 66.5t-64 35t-67 13.5
z" id="x3A6"></path></g><g transform="matrix(.017,-0,0,-.017,12.88,11.25)"><path d="M153 550l-26 -186q79 31 111 31q90 0 141.5 -51t51.5 -119q0 -93 -89 -166q-85 -69 -173 -71q-32 0 -61.5 11.5t-41.5 23.5q-18 17 -17 34q2 16 22 33q14 9 26 -1q61 -50 124 -50q60 0 93 43.5t33 104.5q0 69 -41.5 110t-121.5 41q-53 0 -102 -20l38 305h286l6 -8
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</svg></span></td></tr><tr><td align="left">Ti<sub>41</sub>Zr<sub>25</sub>Be<sub>32</sub>Ag<sub>2</sub></td><td align="center">589</td><td align="center">651</td><td align="center">62</td><td align="center">1148</td><td align="center">0.5131</td><td align="center">0.3748</td><td align="center"><span style="width: 21.1px;"><svg height="11.5125" id="M25" style="vertical-align:-0.17555pt" version="1.1" viewbox="0 0 21.1 11.5125" width="21.1" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.25)"><path d="M488 658v-28q-47 -3 -58.5 -12t-11.5 -39q49 -2 97 -15t93.5 -39.5t73.5 -75t28 -112.5q0 -53 -19.5 -96.5t-50 -71t-70 -47t-77.5 -27.5t-75 -9q0 -36 11.5 -45.5t58.5 -12.5v-28h-223v28q47 3 58.5 12.5t11.5 45.5q-47 1 -94.5 14t-93 39.5t-74.5 76t-29 114.5
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</svg></span></td></tr><tr><td align="left">Ti<sub>41</sub>Zr<sub>25</sub>Be<sub>30</sub>Ag<sub>4</sub></td><td align="center">589</td><td align="center">670</td><td align="center">81</td><td align="center">1107</td><td align="center">0.5321</td><td align="center">0.3950</td><td align="center"><span style="width: 21.1px;"><svg height="11.5125" id="M26" style="vertical-align:-0.17555pt" version="1.1" viewbox="0 0 21.1 11.5125" width="21.1" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,11.25)"><path d="M488 658v-28q-47 -3 -58.5 -12t-11.5 -39q49 -2 97 -15t93.5 -39.5t73.5 -75t28 -112.5q0 -53 -19.5 -96.5t-50 -71t-70 -47t-77.5 -27.5t-75 -9q0 -36 11.5 -45.5t58.5 -12.5v-28h-223v28q47 3 58.5 12.5t11.5 45.5q-47 1 -94.5 14t-93 39.5t-74.5 76t-29 114.5
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</svg></span></td></tr><tr><td align="left">Ti<sub>41</sub>Zr<sub>25</sub>Be<sub>28</sub>Ag<sub>6</sub></td><td align="center">597</td><td align="center">655</td><td align="center">58</td><td align="center">1118</td><td align="center">0.5340</td><td align="center">0.3819</td><td align="center"><span style="width: 29.262501px;"><svg height="11.5125" id="M27" style="vertical-align:-0.17555pt" version="1.1" viewbox="0 0 29.262501 11.5125" width="29.262501" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
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</svg></span></td></tr><tr><td align="left">Ti<sub>41</sub>Zr<sub>25</sub>Be<sub>26</sub>Ag<sub>8</sub></td><td align="center">593</td><td align="center">654</td><td align="center">61</td><td align="center">1153</td><td align="center">0.5143</td><td align="center">0.3746</td><td align="center"><span style="width: 21.1px;"><svg height="11.5125" id="M28" style="vertical-align:-0.17555pt" version="1.1" viewbox="0 0 21.1 11.5125" width="21.1" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
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</svg></span></td></tr><tr class="table-tr"><td colspan="8"><hr class="tbody-hr"/></td></tr></table></td></tr></table>

Thermal parameters of Ti<sub>41</sub>Zr<sub>25</sub>Be<svg height="7.8249998" id="M13" style="vertical-align:-3.25793pt" version="1.1" viewbox="0 0 25.8125 7.8249998" width="25.8125" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
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</svg>Ag<svg height="5.5999999" id="M14" style="vertical-align:-3.21404pt" version="1.1" viewbox="0 0 7.4000001 5.5999999" width="7.4000001" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
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</svg> (<svg height="11.125" id="M15" style="vertical-align:-0.11285pt" version="1.1" viewbox="0 0 37.212502 11.125" width="37.212502" xmlns="http://www.w3.org/2000/svg" xmlns:xlink="http://www.w3.org/1999/xlink">
<g transform="matrix(.017,-0,0,-.017,.062,10.862)"><path d="M536 404q0 -17 -13.5 -31.5t-26.5 -14.5q-8 0 -15 10q-11 14 -25 14q-22 0 -67 -50q-47 -52 -68 -82l37 -102q31 -88 55 -88t78 59l16 -23q-32 -48 -68.5 -78t-65.5 -30q-19 0 -37.5 20t-29.5 53l-41 116q-72 -106 -114.5 -147.5t-79.5 -41.5q-21 0 -34.5 14t-13.5 37
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</svg>, 4, 6, 8 at.%) BMGs. The error of the temperature values is ±1 K.

Advances in Materials Science and Engineering

A Centimeter-Sized Quaternary Ti-Zr-Be-Ag Bulk Metallic Glass

Table 1