Abstract

908 mW of green light at 532 nm were generated by intracavity quasiphase matching in a bulk periodically poled MgO: (PPMgLN) crystal. A maximum optical-to-optical conversion efficiency of 33.5% was obtained from a 0.5 mm thick, 10 mm long, and 5 mol% MgO: crystal with an end-pump power of 2.7 W at 808 nm. The temperature bandwidth between the intracavity and single-pass frequency doubling was found to be different for the PPMgLN. Reliability and stability of the green laser were evaluated. It was found that for continuous operation of 100 hours, the output stability was better than 97.5% and no optical damage was observed.

1. Introduction

Compact and efficient green laser light sources have numerous applications such as laser displays, material processing, biological investigations, and optical communications. There are many methods to achieve coherent green light; however, second harmonic generation (SHG) by the quasi-phase-matching (QPM) technique has been an attractive method to obtain compact and high-efficiency laser [1]. The QPM technique based on periodically poled lithium niobate (PPLN) has significant advantages including phase matching of an arbitrary wavelength by the use of an appropriate period of polarization inversion and a higher nonlinear coefficient than KTP, LBO, and BIBO.

So far, the single-pass SHG scheme is a popular solution for achieving CW green laser light. However, this scheme requires a high nonlinear coefficient and a long interaction length to achieve high conversion efficiency, which can be satisfied by employing PPLN crystals. CW green power of 2.7 W has been obtained in a 50 mm long PPLN single-pass crystal pumped by a 6.5 W Nd:YAG laser [2]. Due to its higher photorefractive damage threshold and lower green-induced infrared absorption as compared with PPLN [3], periodically poled MgO:LiNb (PPMgLN) has replaced the PPLN. A maximum power of 1.18 W at 531 nm with 16.8% conversion efficiency has been obtained from a 2 mm thick, 25 mm long PPMgLN single-pass crystal pumped by a 7 W Nd:GdV laser [4]. Periodically poled Mg-doped stoichiometric lithium tantalate (PPMgSLT) is usually used as an alternative material for high-power generation. 7 W of SHG green light with 35.4% conversion efficiency in a 2 cm long PPMgSLT single-pass crystal pumped by a 19.6 W, 1084 nm Yb-doped fiber laser have recently been reported [5].

Intracavity second harmonic generation (ISHG) of Nd-doped lasers has always been an attractive method for producing green light [6]. Second harmonic generation in a bulk PPLN crystal was demonstrated using the intracavity scheme for the first time in 1995 [7]. In a later experiment, of green ISHG at 541 nm were generated with a pump power of 300 mW, indicating 0.02% optical-to-optical conversion efficiency in 1997 [8]. A maximum output power of 740 mW of blue light has also been generated with an optical-to-optical efficiency of 5.7% at a pump power of 13.5 W [9].

In this paper, we report highly efficient continuous-wave green-light generation based on intracavity frequency doubling, in a quasi-phase-matched PPMgLN bulk crystal. With an end-pump power of 2.7 W at 808 nm, a maximum green output power of 908 mW at 532 nm is achieved with a high optical-to-optical conversion efficiency of 33.5%.

2. Experiments

The experimental setup of a high-efficiency CW, laser-diode (LD), and end-pumped green laser with an intracavity SHG scheme is shown schematically in Figure 1. YV doped with 1% Nd with a size of was used as the gain medium. A 0.5 mm thick, 10 mm long, 2 mm wide, and 5 mol% PPMgLN crystal provided by the C2C Link Corporation, Canada, was used as a frequency doubler. Both sides of the PPMgLN crystal were antireflective (AR), coated at 532 nm and 1064 nm. Temperature of the PPMgLN was controlled by a thermoelectric cooler (TEC).

The laser cavity consisted of a high-reflection (HR) coating at 1064 nm and AR coating at 808 nm on the pumping side of the Nd:YV crystal, as well as a 50 mm radius of curvature mirror (M) with HR coating at 1064 nm and AR coating at 532 nm, which were used, respectively, for folding the fundamental laser beam and for the second harmonic output. The other side of the Nd:YV crystal was AR-coated at 1064 nm and HR-coated at 532 nm. The optical end-pump was a CW-2.7 W-laser diode whose end-face was imaged into the pump side of the Nd:YV crystal by a graded index lens (GRIN). The GRIN with a size of was AR-coated at 808 nm.

3. Experimental Results

The CW green laser output power versus the pump power is shown in Figure 2. To obtain the data, the 808 nm pump LD power was varied by changing the injection current of the LD. When the pump power was up to 2.7 W, the green laser delivered 908 mW with 33.5% optical-to-optical conversion efficiency at . To the best of our knowledge, this is the highest optical-to-optical conversion efficiency reported to date for a green laser at low pump power (<5 W). This conversion efficiency is even higher than that obtained for CW single-pass SHG in a bulk PPMgLN with a 1064 nm pump power of 7 W [4]. It is worth noting that the AR coating of the PPMgLN crystal has not been optimized since multiple beam spots were observed in the far-filed pattern of the green laser. We believe that the efficiency can further be enhanced by optimizing the AR coating conditions.

In order to measure the uniformity of the PPMgLN crystal at different transverse positions, we shifted the PPMgLN crystal transversely when the temperature was set at the phase-matching temperature, while all other conditions are held constant. As shown in Figure 3, change of the green output power is less than 3%, indicating high uniformity of the PPMgLN crystal. Therefore, it is possible that several beams can pass a single PPMgLN crystal at the same time, which can further enhance the optical-to-optical conversion efficiency.

Maximum green output power can be obtained at the phase-matching temperature for PPMgLN crystal. In the previous reports, the single-pass phase-matching temperature has been investigated, but the phase-matching temperature of the PPMgLN in a laser cavity has not been reported. In this paper, the phase-matching temperature of the PPMgLN in the laser cavity was investigated by changing the crystal temperature. As shown in Figure 4, the phase-matching temperature of PPMgLN intracavity frequency doubling is , and the output power is very sensitive to the crystal temperature. The temperature change of could cause nearly 100 mW output drop. In contrast, in the single-pass scheme, the phase-matching temperature is , which is higher than that in the intracavity scheme.

To evaluate the reliability and stability of our green laser, continuous operation for 100 hours was carried out. During that period, no drop in green output power was observed, implying that the photorefractive damage is negligible in our experiments. As shown in Figure 5, the change of the green output power is less than 2.5% for 100 hours, indicating that the PPMgLN crystal is a practical material to use in generating stable green laser light. Longer-time experiment for evaluating the stability of the PPMgLN crystal is in process.

4. Conclusions

CW power of 908 mW at 532 nm with 33.5% optical-to-optical conversion efficiency has been obtained from a 0.5 mm thick, 10 mm long PPMgLN crystal in an intracavity frequency-doubling scheme. It has been shown that the efficiency of the intracavity scheme can be much higher than that of single-pass frequency-doubling scheme, indicating that we can obtain higher efficiency and power by employing the intracavity scheme. At the phase-matching temperature, the output power has shown stable operation for more than 100 hours, and the change of the output power is less than 3% at the different transverse positions of the PPMgLN. The experiment results clearly indicate that practically compact and highly efficient green lasers can be realized based on bulk PPMgLN crystals if the uniformity of the crystal is high. We expect that optical-to-optical conversion efficiency of more than 40% could be achieved if the AR coating of the PPMgLN crystal is improved.

Acknowledgments

The authors thank the C2C Link Corporation for helpful discussion as well as providing the high-quality PPMgLN nonlinear crystal. This work was supported by the Nation High-Tech R&D Program (“863” Program, Contract no. 2006AA030103), the National Key Technologies R&D Program (Contract no. 2006BAK12B13), and the National Knowledge Innovation Program (Contract no. KACX1-11).