Research Article | Open Access

T. Taillandier-Loize, J. Baudon, M. Hamamda, G. Dutier, V. Bocvarski, M. Boustimi, F. Perales, M. Ducloy, "Metaoptics with Nonrelativistic Matter Waves", *Advances in OptoElectronics*, vol. 2012, Article ID 734306, 8 pages, 2012. https://doi.org/10.1155/2012/734306

# Metaoptics with Nonrelativistic Matter Waves

**Academic Editor:**Pavel A. Belov

#### Abstract

The counterpart of metamaterials in light optics for nonrelativistic matter waves governed by the Schrödinger equation can be found by transiently reversing the group velocity using a so called comoving potential. Possible applications to wave-packet dynamics, atom interferometry, and atom deceleration are described.

#### 1. Introduction

The genuine concept of “meta” materials for electromagnetic waves originates from the now famous Veselago’s paper published in 1967 [1]. The basic idea is that, in a material with negative electric permittivity and negative magnetic permeability , Maxwell equations impose that the wave vector **k** and the Poynting vector **S** of a planar wave have opposite directions and, because of causality, the effective optical index is real negative: . The realisation of such artificial or “meta” materials, also called left-handed materials (LHM), in a wide range of wavelengths, has been—and continues to be—the subject of considerable theoretical and experimental efforts [2–4]. Compared to an ordinary material with a positive index, a metamaterial has a similar group velocity, whereas its phase velocity is reversed. This gives rise to the negative refraction phenomenon, owing to which so-called “meta” lenses are conceivable. The concept is rather easily extended to matter waves, provided that the effective mass of the particle be zero or close to zero, as it is the case for electrons in graphene, governed by a (relativistic) Dirac equation [5].

Paradoxically the situation is much more intricate with nonrelativistic particles, as atoms having a thermal velocity (a few hundreds ms^{−1}), the dynamics of which is governed by the Schrödinger equation. The first obstacle is the inability of atoms to penetrate dense matter: hence a “material” should be replaced by a “medium”, namely, some external potential created in vacuum. A second difficulty comes from the fact that, in this situation, the phase velocity is an ambiguous concept since it is gauge dependent and its inversion appears to be problematic, if not meaningless. Nevertheless the key property of a metamedium lies in the opposite directions of phase and group velocities, a property which will be realised in our case by simply reversing the group velocity. Obviously, given a source of atoms, this property has necessarily a transient character since the group velocity is associated to the density of the probability flux which should finally be oriented outwards from the source. As a consequence, the external potential, assumed to depend on a single spatial coordinate (), must be also time dependent, of the type . In the following, the variation in of this potential will be considered as being slow at the de Broglie wavelength () scale, allowing us to use “short wavelength approximations,” for example, WKB or iconal approximation. As shown in part 2, *comoving* potentials [6], of the general form
where is a constant amplitude, is a normalized signal of finite duration, are able to cause the searched inversion of the group velocity and to induce a negative refraction upon the atomic trajectory [7]. The direct observation of this negative refraction on atomic trajectories implies a low velocity and/or a sufficiently high magnitude , that is, in the case of a magnetic potential, a sufficiently intense magnetic field (typically a few hundreds Gauss at a velocity of a few ms^{−1}. An atom interferometer as a Stern-Gerlach interferometer [8] is a much more sensitive tool to evidence the effect, in so far as it transforms a phase shift into a variation of intensity (part 3).

Two other consequences of the group-velocity inversion are worth to be noted: (i) primarily the negative refraction concerns the motion of a wave packet centre, but it affects also the shape of this wave packet, especially its width—which is *reduced*—, along the same general trend, namely, a transient time reversal [9]; (ii) for similar reasons, the fact that the potential is time dependent results into a nonconservation of energy and more precisely (in the case of negative refraction) into a decrease of the atom velocity. This phenomenon plays an important role in atom interferometry. It can be used to slow down atoms (part 4). As the total length of such a slower is an increasing function of the spatial period of the potential, there is a great advantage to make use of a comoving *optical* potential for which is of a few hundreds of nm [10].

Whilst they can give rise to similar effects (together with other specific effects), metamedia for atomic waves are basically different from metamaterials for light optics essentially because of the fundamental difference existing between the related wave equations (Schrödinger versus Maxwell or Dirac). To conclude (part 5), owing to the relative simplicity of their realisation as well as their large domain of applicability, metamedia are expected to play in the future a significant role in atom optics. Nevertheless note that a distinct approach to negative refraction for ultra-cold atoms, based upon “quantum simulators,” allows one to simulate condensed matter physics processes with cold atoms (For instance honeycomb optical lattices may be used to reproduce electron dynamics in grapheme [11, 12]. Also specific non-Abelian gauge potentials, simulated with light fields of given wave-vectors and frequencies allow one to assign a quasi-null effective mass to ultracold atoms ( [13]. Thus, an adequate Klein potential barrier should induce negative refraction.) [11–13]. In the following of this paper we shall not consider this type of situations.

#### 2. General Principle: Negative Index

The concept of comoving field of the form given previously, together with its generic property *to fashion the momentum **-dependence of the resulting phase shift*, have been introduced in 1997 [6]. Indeed it can be shown [10], using the WKB approximation, that for a field differing from zero within a given interval [], an incident plane wave of specific momentum , freely propagating along the direction , is altered by the comoving potential *via* a simple phase factor, becoming with
In (2), ], is smaller than and arbitrarily close to , is the atom mass and the Heaviside function. The second term in (2) results from the time-dependence of , hence the nonconservation of energy. It warrants the continuity of and and their derivatives at .

Let us now consider a wave packet, the momentum distribution of which, , is centred at . Using the stationary-phase approximation, it is seen that the potential induces a spatial shift upon the motion of the wave packet centre:
which gives:
For , the integral part takes a finite limiting value, whereas the other term, linear in (), corresponds to a definite change
of the final velocity. This change becomes negligible for comoving pulses of a sufficiently long duration, provided that the product ) tends to zero when . The important point here is that, by a proper choice of , the -dependence of can be made such that the group velocity (i.e., the velocity of the wave packet centre) be transiently negative. A trajectory initially in plane , with initial velocity components , , remains in this plane, exhibiting the negative refraction since becomes transiently negative whereas the motion along remains unaltered. For a sufficiently large value of , the behaviour of the trajectory is similar to that of a ray traversing a negative-index flat plate with parallel surfaces. Figure 1(a) shows an example of such a trajectory for a metastable argon atom Ar*(^{3}P_{2}), spin polarized in Zeeman state , experiencing a magnetic comoving potential with being the Landé factor, the Bohr magneton and mT the magnetic field intensity. In this example, mm, m s^{−1}, m s^{−1}. The time-dependent signal is with and . Note that, at these low velocities, the lateral shift of the trajectory is rather large (1.2 mm) in spite of the relatively modest value of the magnetic field. Other values of would lead to shifts proportional to , which means that the comoving potential acts as an efficient beam splitter. More generally the comoving potential zone behaves as a multirefringent plate.

**(a)**

**(b)**

**(c)**

Assuming that deflection angles are small, by comparison with the light-optics counterpart under similar conditions, one can obtain an effective index given, for , by [14]
where is an estimate of the time at which reaches its asymptotic value (). As it is seen in Figure 1(b), for , the effective index becomes negative for values of larger than a critical value, mT in the present case. The fact that at is not really a singularity since it simply means, in the light-optics analogy, that the ray inside the plate is normal to the plate’s surfaces. On the other hand, for , is positive for any value of , giving rise to ordinary positive refraction. The effective index given by (6a) is a constant related to a simplified trajectory consisting of three portions of straight lines. In the case of a comoving field, on the other hand, the index is -dependent. It can be derived from the usual ray equation in an inhomogeneous medium: (**r**′)′ = , where being the curvilinear abscissa. As a function of the variable , the element of curvilinear abscissa is . Then the index is simply:
where is a constant such that . This expression of n simply reflects the Snell-Descartes refraction law in a medium stratified by planes orthogonal to , namely

where = ArcTan. Finally, once modelled the trajectory, the index profile can be derived. Note that has the sign of and, as expected, it is infinite when . Actually especially at large values of , the index profile derived from ((6b)-(6c)) depends on the angle of incidence since the constant in (6c) is . On the other hand the medium is invariant in any translation along . As a conclusion the metamedium is *anisotropic*. Figure 1(c) shows the 2D profile of the index derived from an ensemble of trajectories similar to that of Figure 1(a), but calculated with different incidence angles ranging from 0 to 0.1 rad.

#### 3. Negative-Index Medium in a Stern-Gerlach Atom Interferometer

A standard Stern-Gerlach atom interferometer [8], also called some years later “spin-echo experiment,” in analogy to the well-known method of neutron spin-echo [15, 16], is a longitudinal polarisation interferometer in which an integrable static magnetic field profile , that is, a -dependent magnetic potential , induces upon a planar wave (of momentum ) describing the external motion along , a phase shift of the form . In the following semiclassical approximation:
where . Starting from a given Zeeman state issued from a polarizer, for example, a Stern-Gerlach polarizer, one first prepares, using Majorana transitions (fast rotation of a tiny magnetic field) [17], a linear superposition of -states
where the are constant coefficients. Beyond the field profile , it becomes
Then a second Majorana zone generates the new combination (where the -s are constant)
Finally, an analyzer (similar to the polarizer) selects a specific Zeeman state and one measures the final intensity
It contains interference terms in which can be evidenced by varying the magnitude of the magnetic field or the velocity. In place of a static field profile, a comoving field can be used as well, as it has been demonstrated in [6] with a beam of fast ( ms^{−1}) metastable hydrogen atoms (2, ). Very recently, experiments dealing with similar questions have been realized by Sulyok et al. with a beam of neutrons at a velocity of 2000 ms^{−1}, in a so-called perfect crystal interferometer [18]. The magnetic potential they use is a sum of terms of the form , where is a square function of a definite width and , , are constants. It might seem different from our comoving potential. However it can be readily seen (by taking the Fourier transform of the spatial dependence) that this potential is actually a sum of comoving terms.

The main questions that arise about the use of comoving potentials as phase objects in an interferometer deal with similarities and differences they present with respect to static potentials. The first specificity of comoving potentials is that, because of the transient character of the effect, a treatment using wave packets is needed. Apart from the narrowing effect mentioned previously (difficult to observe except at low velocity), the first consequence of that is the *critical velocity dependence* of the interference effect, particularly when a purely sinusoidal signal of the type is used. Indeed in that case there exists a “resonant” atomic velocity coinciding with the field velocity . This resonant velocity can correspond to a bright fringe or a dark fringe, according to the value of the magnitude of the magnetic field (which is generally low, less than 100 mG). This central fringe is surrounded by few other fringes within the envelope of the resonance. This phenomenon has been observed using a time-of-flight technique, with a single zone (see Figure 2, taken from [6]) or a double zone of comoving field.

Another manifestation, specific of comoving potentials, appears when a nonsinusoidal signal of a finite duration is used, for example, for elsewhere. When the value of the cut-off time is large compared to , final velocities and related to sublevels and , are almost equal to the initial velocity . On the contrary, when is comparable to or smaller than , one gets (beginning of a negative refraction) and . At , the abscissas of the “+” and “−” wave packets are such that , then their mutual longitudinal separation monotonously increases with or , which cancels any interference effect between them (once remixed), in other words a total loss of contrast as the distance to the detector is increased. Figure 3(a) shows as a function of in the realistic case of metastable argon atoms of initial velocity 560 m s^{−1}. Whilst the magnitude of may seem small (a fraction of 1 *μ*m), it is much larger than the wavelength (0.02 nm) and the effect on the interference is drastic. A similar phenomenon is described in [18] for the case of neutron interferometry. In principle it is possible to recover the contrast *via* the action of a second reversed comoving pulse provided that the characteristics of this second pulse (especially its duration ) are adjusted such that the final velocities are exactly equal to each other. Figure 3(b) shows an example of such compensation—over a distance of several centimetres—by means of a second reversed pulse similar to the first one but applied 2 ms later.

**(a)**

**(b)**

Figure 4 shows the high sensitivity of the interferometer operating with metastable argon atoms at thermal velocity (560 ms^{−1}). At such large velocity the inelastic effect induced by the potential pulse is small enough to make the contrast practically independent of the distance at which the detector is placed (from 0.1 to 1 m). On the other hand the contrast is reduced at “large” field magnitude, of the order of 0.1 mT or more, because of the increasing spatial separation between the two interfering wave packets and the related decrease of their overlap.

#### 4. Atom (or Molecule) Slower

As explained in part 2, the primary effect of a potential pulse, comoving in the direction, the sign of which is such that (for a sufficient magnitude) it results into a negative refraction, is to reduce the velocity component along by an amount, derived from (3) (for ):
In principle this effect can be used to slow down atoms or molecules. For neutrons this was shown to work [19]. However when the initial velocities are in the thermal range (e.g., 560 ms^{−1} for Ar* atoms) the predicted reduction of is quite small, typically of a few mm s^{−1}, at least (in the case of a magnetic potential) for reasonable values of , namely less than 0.1 T. As a consequence, to reduce the velocity down to almost zero, a large number of successive pulses is needed. This is made possible by the fact that, immediately after the end of a pulse of duration the velocity is practically equal to the reduced velocity obtained at time . Then, when (after a short blank) the next pulse is applied, this latter velocity becomes the initial velocity, which is in turn reduced, and so forth. The best choice for the pulse duration is such that derived from (5) takes its first maximum value. For a signal of the form [6], there exists an optimum value of the time constant leading to an absolute maximum of . For ms^{−1}, the best values are obtained for and . Actually they are almost equal to each other and their dependence on is such that the product of the optimum value of by is a constant. This means that the atomic path covered through successive pulses is almost a constant.

The present method bears some similarities with the so-called “adiabatic slowing” [20, 21]. This latter method has been applied to a wide variety of species, such as hydrogen atoms, polar and non polar molecules [22], Rydberg atoms and Rydberg molecules [23–25]. Low final velocities (a few 10 ms^{−1}) are accessible, but at the price of rather strong fields (e.g., in [23–25]). Here, the nature of the force is quite different, since it derives from a special potential depending on both space and time. In principle the method is applicable to the same species, with the advantage that it uses much lower fields.

As shown in [10] an atom slower using magnetic potential pulses (, mm) is able to reduce the velocity of metastable argon atoms from 560 m s^{−1} down to almost zero over a distance of 2.2 m, comparable to the total length of a standard Zeeman slower [26]. For a given magnitude of the potential, the length is governed by the spatial period . In a simple magnetic version, it is almost impossible to reduce it below 1 mm, whereas the use of a dipolar *optical* potential obtained in a off-resonance standing wave provides us with a huge reduction of the period, which is half the optical wavelength /2 (in the case of metastable argon atoms). Far from resonance the general form of such a potential is [27]:
where Ω is the Rabi frequency and the detuning. To operate “far from resonance” (to avoid any spontaneous emission), the difference between the laser frequency and the two resonances appearing in the standing wave, Doppler-shifted by , must be large compared to the power-broadened line width , where is the natural line width and Σ the saturation parameter. To get a magnitude of the potential sufficiently high to achieve the complete slowing over a distance shorter than say, 20 cm, using a reasonable laser power (e.g., 32 mW mm^{−2}), a moderately large (negative) detuning should be chosen, such as = −23*.*45 × 10^{9} rad/s (3*.*45 GHz). This leads to a ratio , large compared to 1. As the velocity is lowered, Δ decreases, tending to zero as . Then either the detuning is kept constant and the condition is better and better verified, or is kept equal to 5Δ, allowing us to reduce the intensity (as ) as well as (as ), but then the ratio R decreases as , which implies a lower limit for ( at ). As before a series of many pulses separated from each other by small blanks is applied, each of them (numbered ) providing a small decrease of the velocity (a few mm/s). The duration of each pulse is adjusted in such a way that the first maximum value of is reached at the end of the pulse. As previously the path covered by the atom during successive pulses is roughly a constant (*≈*0*.*12 m). Figure 5 shows how the velocity decreases down to almost zero (with the restriction mentioned before) as a function of . The total number of applied pulses is large (about 2 10^{6}) but the total length is now 19.2 cm. Note that the method does not imply any permanent magnetic moment of the atom and is applicable for instance to Ar*(^{3}P_{0}) metastable atoms.

In addition to the advantages of its short length and the absence of any random spreading of the velocity (at least if the spontaneous emission is negligible), the present decelerator is interesting from the point of view of the atomic density in the phase space. Indeed an important characteristic of comoving fields is their effect on the longitudinal spatial width of the atomic wave-packet. As mentioned previously [9], comoving potentials are able to transiently narrow wave packets, compensating for the free-propagation natural spreading. In the present case this effect is very small at the beginning of the deceleration process but becomes more and more important as the velocity decreases. As a result the wave packet width progressively deviates from the free-propagation width to rejoin its initial value (0). On the other hand it can be verified, using the Wigner function, that the width of the momentum distribution remains unchanged, the reason being that the effect of the potential is a pure real phase shift. Consequently the density ()^{−1} in the phase space (), instead of continuously decreasing, recovers its initial value at the end of the slowing process.

#### 5. Conclusion

In this paper comoving fields have been introduced in view of realizing negative-index media for matter waves in the nonrelativistic regime. Because of the fundamental difference between Schrödinger and Maxwell (or Dirac) equations, especially for what concerns the phase velocity, a method quite different from those used in light optics or ultrarelativistic particle optics is needed. The aim of our method is the transient inversion of the group velocity. Phenomena similar to those observed in metamaterials, as the negative refraction, metalens, etc.) are expected. Other properties are specific of our “meta-media.” In particular, the evolution of the wave-packet spatial width exhibits unusual features, as a transient narrowing, accompanying the negative refraction and related to time reversal, and also a velocity change in the case of short comoving potential pulses because of the nonconservation of energy.

All these effects, on atom trajectories or wave-packet width evolution, are directly observable provided that the atomic velocities are low, typically of a few ms^{−1}. At higher velocity, like a few hundreds of ms^{−1}, more sensitive techniques are necessary. Atom interferometers in general and Stern-Gerlach interferometers in particular, offer such sensitivity. We have shown that observable optical-index effects appear with magnetic fields as small as a few T.

We have proposed an approach to atom beam deceleration based on dispersive optical forces. Atom stopping should be almost achieved on short distances using a moderate laser power, for example, less than 50 mW/mm^{2}. The absence of spontaneous emission processes should allow preservation of the transverse coherence properties of the initial beam. The technique is especially applicable to narrow supersonic beams, like metastable rare-gas atom beams, and it is able to provide us with ultra-low-velocity beams for coherent atom optics and atomic interferometry. It is also a promising technique applicable to slowing down not solely diamagnetic atoms (such as metastable argon atoms in the ^{3}P_{0} state) but also molecules since any optical pumping toward molecular levels other than those interacting with light is absent. Slowing and trapping of molecules is a subject of a particular importance in the investigation of cold collisions (determination of intermolecular potentials at large distances, resonances of various kinds).

#### Acknowledgments

The authors from Laboratoire de Physique des Lasers acknowledge the Institut Francilien de Recherche sur les Atomes Froids (IFRAF) for support.

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#### Copyright

Copyright © 2012 T. Taillandier-Loize et al. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.