Table of Contents
Laser Chemistry
Volume 19 (1999), Issue 1-4, Pages 41-44

Resonance Raman and Optical Dephasing Study of Hitci

Max-Born-Institut, Rudower Chaussee 6, Berlin D-12474, Germany

Received 7 April 1997

Copyright © 1999 Hindawi Publishing Corporation. This is an open access article distributed under the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.


Line shape analysis based on resonance Raman spectra of HITCI is used to determine the details of the vibrational part of the line broadening function. Forced Light Scattering with 20 fs pulses from a Ti: sapphire laser measured optical dephasing probing with an Ar+ laser. The observed response is well described by the line broadening function derived from the fluorescence line shape.