Abstract

Combining the propagation model of guided waves in a multilayered piezoelectric composite with the interfacial model of rigid, slip, and weak interfaces, the generalized dispersion characteristic equations of guided waves propagating in a piezoelectric layered composite with different interfacial properties are derived. The effects of the slip, weak, and delamination interfaces in different depths on the dispersion properties of the lowest-order mode ultrasonic guided wave are analyzed. The theory would be used to characterize the interfacial properties of piezoelectric layered composite nondestructively.

1. Introduction

The acoustic wave propagation in piezoelectric materials has received considerable attention from engineering and scientific communities involved in nondestructive evaluation and transducer design. Numerous ultrasonic devices using piezoelectric materials are currently being developed for a variety of applications, such as SAW filters, ultrasonic transducers, and a variety of physical, chemical, and biological sensors [1, 2]. In aerospace and other structural applications, piezoelectric layered smart or intelligent composites are being used [3]. Many of these applications involve layered structures made up of piezoelectric materials.

Layered composite materials are usually made of different materials. Very thin adhesive interfacial layer serves as the bonding between adjacent layers. Some imperfections, such as cracks and small voids, often emerge at the interface and contribute to the fatigue of the composite. The interfacial property between layers is one of the key factors that determine the structural stability of composites. It is, therefore, very important to characterize the adhesive layer quality, which has been a main topic in nondestructive testing and evaluation of composite materials [48].

Ultrasonic wave is a mechanical wave, which reflects the elastic properties of the medium. The interfacial mechanical property is closely related to the coupling strength between layers in the structure and the level of acoustic impedance match between the bonding layer and the piezoelectric material. Because of its deep penetration ability, ultrasonic technique is among the most promising nondestructive evaluation methods for the interfacial layer characterization. There are some papers considering the wave propagation in this structure with perfect interface, that is, the stress and displacement across the interface are continuous [911].

This paper is concerned with the guided waves propagating in piezoelectric layered composite with different interfacial properties. First, the transfer matrix of the piezoelectric layer is derived. Then, based on the model of piezoelectric layered composite, the general dispersion equations of the guided waves propagating in it with rigid, slip, and weak interfaces are presented by using the transfer matrix techniques. Numerical analysis has been performed on typical Y-cut, Z-propagating lithium niobate multi-layered composite with slip, weak, and delamination interface in different depth. It is shown that the interface property and the interfacial defect depth have strong effect on the guided wave phase velocity. The theoretical work in this paper is intended to provide fundamental principles in nondestructive testing and evaluation of the interface of piezoelectric layered composite.

2. Transfer Matrix of Piezoelectric Layer

The transfer matrix method has long been used in modeling multi-layered structures [12]. The transfer matrix expresses the relationship of characterized parameters between the top and the bottom interface of a layer. The order of transfer matrix is determined by parameters of the layer material. To a piezoelectric layer, the transfer function consists of an 88 matrix. Figure 1 shows the labeling system used in this paper. The waves propagate along the 𝑥1 direction of a piezoelectric layer with its poling direction along 𝑥3. We consider a two-dimensional problem assuming all field components are constant in the 𝑥2 direction.

In the piezoelectric plate, the coupled wave equations using the quasistatic approximation are𝜌𝜕2𝑢𝑗𝜕𝑡2𝑐𝑖𝑗𝑘𝑙𝜕2𝑢𝑘𝜕𝑥𝑖𝑥𝑙𝑒𝑘𝑖𝑗𝜕2𝜙𝜕𝑥𝑖𝑥𝑘𝑒=0,𝑖𝑘𝑙𝜕2𝑢𝑘𝜕𝑥𝑖𝑥𝑙𝜀𝑖𝑘𝜕2𝜙𝜕𝑥𝑖𝑥𝑘=0,(1) in which 𝜌 is the density of material, 𝑢𝑘 is the particle displacement vector, and 𝜙 is the electric potential. 𝑐𝑖𝑗𝑘𝑙, 𝑒𝑖𝑗𝑘, and 𝜀𝑖𝑘 are, respectively, the tensor components of the elastic stiffness measured at constant electric field, the piezoelectric constant, and the dielectric permittivity measured at constant strain. The subscripts 𝑖,𝑗,𝑘, and 𝑙 range over the values 1, 2, and 3, and the summation convention on repeated subscripts is employed. The solution of the form is assumed as𝑢𝑗=𝛼𝑗exp𝑖𝑘𝑏𝑥3𝑥exp𝑖𝑘1,𝑣𝑡𝜙=𝛼4exp𝑖𝑘𝑏𝑥3𝑥exp𝑖𝑘1,𝑣𝑡(2) where 𝑏 is the attenuation coefficient. Substituting (2) into (1), we obtainΓ𝑖𝑗𝛿𝑖𝑗𝜌𝑣2𝛼𝑗=0,(3) where 𝑣 is the phase velocity of the wave. The symmetric matrix Γ is given byΓ𝑖𝑗=𝑐3𝑖3𝑗𝑏2+𝑐1𝑖3𝑗+𝑐3𝑖1𝑗𝑏+𝑐1𝑖1𝑗,Γ𝑖4=𝑒3𝑖3𝑏2+𝑒1𝑖3+𝑒3𝑖1𝑏+𝑒1𝑖1,Γ44𝜀=33𝑏2+𝜀13+𝜀31𝑏+𝜀11.(4) Equation (3) has a nontrivial solution only if ||Γ𝑖𝑗𝛿𝑖𝑗𝜌𝑣2||=0.(5) For every value of 𝑣, (5) has eight eigenvalues of 𝑏. There are also eight four-component eigenvectors corresponding to the eight eigenvalues. Thus, the general solution can be written as𝑢𝑗=𝑛𝐶𝑛𝛼𝑗(𝑛)exp𝑖𝑘𝑏(𝑛)𝑥3𝑥×exp𝑖𝑘1,𝑣𝑡𝜙=𝑛𝐶𝑛𝛼4(𝑛)exp𝑖𝑘𝑏(𝑛)𝑥3𝑥×exp𝑖𝑘1,𝑣𝑡𝑛=18,(6) where 𝐶𝑛 is the weighting coefficients.

The normal components of stress and electric displacement of piezoelectric materials are𝜎3𝑗=𝑐3𝑗𝑘𝑙𝜕𝑢𝑘𝜕𝑥𝑙+𝑒𝑘3𝑗𝜕𝜙𝜕𝑥𝑘,𝐷3=𝑒3𝑘𝑙𝜕𝑢𝑘𝜕𝑥𝑙𝜀3𝑘𝜕𝜙𝜕𝑥𝑘.(7)

Assume that the displacement, stress, electric displacement, and potential are known at the top interface of the plate. According to (6) and (7), the weighting coefficients can be written as𝐶1𝐶2𝐶3𝐶4𝐶5𝐶6𝐶7𝐶8=[𝑀]1top𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙top.(8)

At the bottom interface, the displacement, stress, electric displacement, and potential are𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙bottom=[𝑀]bottom[𝑀]1top𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙top.(9) The matrix product in this equation now relates the characterized parameters between the top and the bottom interface of a piezoelectric layer and is defined as the transfer matrix [𝑃],[𝑀]bottom[𝑀]1top=[𝑃].(10)

3. Wave Equations in Piezoelectric Layered Composite

The model and the coordinate system of the piezoelectric layered composite are shown in Figure 1. Waves propagate along the 𝑥1 direction. In the transfer matrix method, the intermediate interfaces are eliminated so that the fields in all layers are described solely in terms of external boundary conditions. The displacement, stress, electric displace, and potential must be continuous across a rigid interface between two layers; 𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙𝑗+1,top=[𝑃]𝑗𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙𝑗,top.(11) This process can be continued layer by layer, resulting in the follwing equation;𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙𝑛,bottom=[𝑄]𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙1,top,(12) where 𝑛 is the last layer and [𝑄] is the system matrix consisting of the matrix product of layer matrices;[𝑄]=[𝑃]1[𝑃]2[𝑃]𝑛1[𝑃]𝑛.(13) The wave must satisfy the appropriate electrical and mechanical boundary conditions on both surfaces of the composite. The top and bottom of composite are free. So the normal stresses at the extreme interfaces (top and bottom) must be zero. Then the mechanical boundary conditions are𝜎31𝑛,bottom=𝜎311,top𝜎=0,(14)32𝑛,bottom=𝜎321,top𝜎=0,(15)33𝑛,bottom=𝜎331,top=0.(16) The metallization on plate surfaces is assumed to consist of a perfectly conducting film of negligible thickness. Thus, the presence of the metal film does not alter the mechanical boundary conditions. However, the electrical boundary conditions vary according to whether it is open (unmetallized) or shorted (metallized). We consider the case where both surfaces are open circuit condition. The electrical boundary conditions are𝐷3𝑛,bottom=𝑘𝜀0[𝜙]𝑛,bottom,𝐷(17)31,top=𝑘𝜀0[𝜙]1,top,(18) where 𝜀0 is the dielectric constant of the vacuum. According to (14)–(17), (12) can be written as[𝐴]𝑢1𝑢2𝑢3𝜙1,top[𝐴]=𝑄=0,41𝑄42𝑄43𝑄481+𝑘𝜀0𝑄51𝑄52𝑄53𝑄581+𝑘𝜀0𝑄61𝑄62𝑄63𝑄681+𝑘𝜀0𝑄71𝑘𝜀0𝑄81𝑄72𝑘𝜀0𝑄82𝑄73𝑘𝜀0𝑄83𝑄78𝑘𝜀0𝑄881+𝑘𝜀0.(19)For this equation to be satisfied, the submatrix must be singular, ||𝐴||=0.(20) Equation (20) is the dispersion equation of the piezoelectric layered composite with rigid interfacial condition.

If there is a slip interface between the 𝑗th and the (𝑗+1)th layers, the interface can only transfer normal displacement and stress. The normal displacement and stress of two layers are continuous, and the shear stresses are zero. So the interfacial boundary conditions are𝑢3𝑗,bottom=𝑢3𝑗+1,top,𝜎31,𝑗,bottom𝜎=0,31𝑗+1,top𝜎=0,32𝑗,bottom𝜎=0,32j+1,top𝜎=0,33j,bottom=𝜎33j+1,top,𝐷3j,bottom=𝐷3j+1,top,[𝜙]j,bottom=[𝜙]𝑗+1,top.(21) The other interfaces of the composite are all rigid, therefore𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙𝑛,bottom=[𝐷]𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙𝑗+1,top,(22) where[𝐷]=[𝑃]𝑗+1[𝑃]𝑗+2[𝑃]𝑁1[𝑃]𝑛,𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙𝑗,bottom=[𝐸]𝑢1𝑢2𝑢3𝜎31𝜎32𝜎33𝐷3𝜙1,top,(23) where[𝐸]=[𝑃]1[𝑃]2[𝑃]𝑗1[𝑃]𝑗.(24) By combining (22)–(24) with (21), the dispersion equation of the piezoelectric layered composite with a slip interfacial condition becomes||||||||||||𝐷41𝐷42𝐹11𝐹12𝐷51𝐷52𝐹21𝐹22𝐷61𝐷62𝐹31𝐹32𝐷71𝐷72𝐹41𝐹42||||||||||||=0,(25) where𝐹11𝐹12𝐹21𝐹22𝐹31𝐹32𝐹41𝐹42=𝐷43𝐷46𝐷47𝐷48𝐷53𝐷56𝐷57𝐷58𝐷63𝐷66𝐷67𝐷68𝐷73𝐷76𝐷77𝐷78𝐸31𝐸32𝐸33𝐸38𝐸61𝐸62𝐸63𝐸68𝐸71𝐸72𝐸73𝐸78𝐸81𝐸82𝐸83𝐸88𝐺100111𝐺12𝐺21𝐺22,𝐺11𝐺12𝐺21𝐺22=𝐸43𝐸48𝐸53𝐸581𝐸41𝐸42𝐸51𝐸52.(26) The rows 1 to 6 and 8 of the matrix [𝐷] are the same as those of matrix [𝐷]. The row 7 of matrix [𝐷] satisfies𝐷7𝑗=𝐷7𝑗𝑘𝜀0𝐷8𝑗.(27) The columns 1 to 6 and 8 of matrix [𝐸] are the same as those of matrix [𝐸]. The column 7 of the matrix [𝐸] satisfies𝐸𝑗7=𝐸𝑗7+𝑘𝜀0𝐸𝑗8.(28) If there is a weak interface between the 𝑗th and the (𝑗+1)th layers, the “spring” model can be used to characterize the interface property [13, 14]. So the interfacial boundary conditions are𝜎33𝑗,bottom=𝜎33𝑗+1,top=𝐾𝑛𝑢3𝑗,bottom𝑢3𝑗+1,top,𝜎31𝑗,bottom=𝜎31𝑗+1,top=𝐾𝑡1𝑢1𝑗,bottom𝑢1𝑗+1,top,𝜎32𝑗,bottom=𝜎32𝑗+1,top=𝐾𝑡2𝑢2𝑗,bottom𝑢2𝑗+1,top,(29) where 𝐾𝑛, 𝐾𝑡1, and 𝐾𝑡2 are the normal stiffness coefficient, the shear stiffness coefficient of the 𝑥1-dimension and 𝑥2-dimension, respectively.

The dispersion equation of the piezoelectric layered composite with a weak interfacial condition is given by||||||||||||𝑍41𝑍42𝑍43𝑍48𝑍51𝑍52𝑍53𝑍58𝑍61𝑍62𝑍63𝑍68𝑍71𝑍72𝑍73𝑍78||||||||||||=0,(30) where[𝐻]=1100𝐾𝑡1100000100𝐾𝑡2100000100𝐾𝑛,[𝑍]=[𝐷]000001000000001000000001000000001000000001[𝐻][𝐸].(31)

4. Numerical Results and Discussion

The analysis presented in the previous section has been applied to calculate the characteristics of the 𝐴0 and 𝑆0 modes propagating in a Y-cut, Z-propagating lithium niobate layered composite. The material constants of the LiNiO3 come from [15]. Since this paper deals with the effect of the interfacial properties of composite on the dispersion characteristics of the guided waves propagating, it is assumed that each layer has the same material, crystal type, cut direction, and thickness. The piezoelectric plate has 40 layers, and the thickness of each layer is 25 μm. In this paper, the structure with a defective interface is represented as m/n. The left and right number of the symbol “/” represent the number of layers on and under the defective interface.

Figure 2 shows the Lamb wave phase velocities of the 𝐴0 and 𝑆0 modes as a function of frequency with a delamination interface in different depth. The dispersion characteristic of 𝐴0 and 𝑆0 modes in an YZ LiNiO3 plate looks very similar to that of the lowest order Lamb waves propagating in a plate of isotropic plate [16]. However, It should be noted that 𝐴0 and 𝑆0 modes in piezoelectric composite have all three components of particle displacement, that is, the waves are more general Lamb waves. As the frequency increases, the 𝐴0 and 𝑆0 mode velocities tend asymptotically to the SAW velocity. Further, it can be shown that the phase velocity of the 𝐴0 mode increases when the depth of the delamination interface increases while the phase velocity of the 𝑆0 mode decreases when the depth of the delamination interface increases. Figure 3 shows the Lamb wave phase velocity of the 𝐴0 mode as a function of frequency with a slip interface in different depth. Except for the 20/20 structure, the phase velocity does not tend asymptotically to a constant velocity when the frequency increases. If the frequency less than 2.5 MHz is considered, the phase velocity of the Lamb wave decreases with the depth when it is less than one-half of the plate thickness, but increases with the depth when it is more than one-half of the plate thickness.

When the interface is weak, the stiffness 𝐾𝑛 and 𝐾𝑡𝑖 are finite values. Figure 4 shows the Lamb wave phase velocity of the 𝐴0 mode as a function of frequency with a weak interface in different depth. It is assumed that 𝐾𝑛 and 𝐾𝑡2 are infinite, and that 𝐾𝑡1 is 5 × 1015 N/m3. Like the condition of the slip interface, the phase velocity does not show saturation when the frequency increases, except for the 20/20 structure. From Figures 3 and 4, one can find that the dispersion characteristic with a weak interface is between that of a slip interface in the same depth and that of the ideal rigid interface. Furthermore, the dispersion characteristic with a weak interface in the central plate is the same as that of a slip interface.

Figure 5 shows the 𝐴0 mode phase velocity versus the defect depth at 1 MHz. When the central interface of the composite has a delamination interface, the phase velocity is the same as that when it has a slip interface. When the depth of the delamination interface is less than half of the thickness of the composite, the phase velocity is less than that of a slip interface in the same depth, and vice versa. The phase velocity with a delamination and slip interface is less than that with a weak interface in the same depth.

Figure 6 presents the effect of the interface stiffness constants 𝐾𝑡1on the phase velocity of the 𝐴0 mode in the 10/30 composite structure. In the calculation 𝑓 is equal to 1 MHz, and 𝐾𝑛 and 𝐾𝑡2 are infinite. It reveals that the phase velocity of the 𝐴0 mode increases with the increasing 𝐾𝑡1. When 𝐾𝑡1 approaches zero, the phase velocity approaches that of a composite with a slip interface. When 𝐾𝑡1 approaches infinity, the phase velocity approaches to that of a composite with a rigid interface. Very large variation of the phase velocity of the 𝐴0 mode can be seen when 𝐾𝑡1 varies in the range of 1012–1015 N/m3.

Figure 7 shows the Lamb wave phase velocity of the 𝑆0 mode as a function of frequency with a rigid, slip, and weak interface in the 10/30 composite structure. Unlike 𝐴0 mode, the interface properties have very little effect on the phase velocity of 𝑆0 mode.

5. Conclusions

We have conducted a theoretical investigation of the velocity variation of guided waves propagating in piezoelectric multi-layered composite with different interfacial properties. General dispersion equations for a composite that contains rigid, slip, and weak interfaces are derived by using the transfer matrix technique. The phase velocities of the lowest antisymmetry and symmetry modes have been numerically computed on a YZ lithium niobate layered composite with slip, weak, and delamination interface in different depth. As the depth of the defective interface changes, the velocity of the lowest anti-symmetry mode changes drastically. But the velocity of the lowest symmetry mode is almost not effected by the interface characteristics. When the interface stiffness coefficient varies in the range of 1012–1015 N/m3, the velocity of the lowest anti-symmetry mode has the largest change.

Acknowledgments

This paper is supported by the National Natural Science Foundation of China (10904073), the Natural Science Research Project of Jiangsu Higher Education Institutions (10 KJB510011), and the Priority Academic Program Development of Jiangsu Higher Education Institutions.